Define backtab with general, and override org-mode indentation function in evil insert mode!

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(general-def 'normal "<backtab>" 'jr/evil-close-fold) Not sure I understand your second question correctly. Let me know if this was not what you are looking for. You can use `org-cycle` in place of `evil-toggle-fold` also. (general-def 'insert org-mode-map "<tab>" 'evil-toggle-fold)